2026,
13(5):
1041-1053.
doi: 10.1109/JAS.2026.125945
Abstract:
Accurate estimation of electrochemical states serves as a pathway to observe internal battery behaviors, effectively bridging the gap between micro mechanism and macro performance and enabling more precise control in an advanced battery management system. Yet conventional pseudo-two-dimensional (P2D) physics methods suffer from high computational complexity and limit their online application. Thus, we develop a model-informed neural network (MINN) framework that synergistically combines deep learning with a physics-based model to accurately monitor the battery electrochemical state (such as lithium-ion concentration, plating potential). Firstly, the MINN model is constructed with the innovative loss term containing experimentally measurable parameters and governing physical laws. Secondly, a composite framework based on a convolutional neural network (CNN) architecture is integrated to automatically extract features and enforce spatial boundary conditions, which significantly reduces the number of boundary loss terms that need to be solved and alleviates the complexity of the training process. After training, the MINN model can achieve an accurate estimation of internal states and even their spatiotemporal distributions that cannot be directly measured based on limited observable data and physical laws. At last, by incorporating dynamic current input, the well-trained basic model exhibits strong robustness and can be directly transferred to other cycling protocols with high accuracy, requiring no further retraining. MINN is a novel and promising framework to realize online and accurate micro electrochemical states monitoring, achieving at least 776 times speedup compared with the P2D model. As an innovative artificial intelligence assisted modeling for electrochemical systems, this framework enables root-cause analysis of battery behavior and failure modes, while empowering the management system with more reliable and trustworthy decision-making capabilities.
Y. Zhang, Q. Zhang, B. Duan, P. Gu, C. Li, and C. Zhang, “Perceiving the battery multi-electrochemical states in real-time based on model-informed neural network,” IEEE/CAA J. Autom. Sinica, vol. 13, no. 5, pp. 1041–1053, May 2026. doi: 10.1109/JAS.2026.125945.